You can do it with:
var queryableResultItems = context.GetQueryable<GlobalSearchResultItem >()
.Where(expression)
.OrderByDescending(x => x["termfreq(content_t, \""+ term+ "\")"])
But I suggest you to setup logic that you need on Solr side. Sorl sorts the results based on the basis of the relevancy of the term present in the field OOTB (it uses tf-idf algorithm to calculate scoring).
You should check query analizer forof your field type in managed-schema (your field should be tokenized):
<analyzer type="query">
<tokenizer class="solr.WhitespaceTokenizerFactory"/>
...
</analyzer>
You can check it in Solr by adding "score" in fl textbox. You can also see how scoring is calculating by checking debugQuery: